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Charleroi is a borough in Washington County, Pennsylvania, along the Monongahela River, 25 miles south of Pittsburgh. Charleroi was settled in 1890 and incorporated in 1891. The population in 1900 stood at 5,930; in 1910, 9,615; in 1920, 11,516, and in 1940, 10,784. The population was 4,871 at the 2000 census.

There has been a large-scale cessation of industrial activities in the region. The decrease in the population is associated with the decline of the steel-making industry in the "Mon Valley" which extends from Charleroi to the mouth of the Monongahela at Pittsburgh.

Charleroi is located at 40°8′17″N, 79°54′5″W (40.138088, -79.901333)^GR1.

According to the United States Census Bureau, the borough has a total area of 0.9 square miles (2.2 km²), of which, 0.8 square miles (2.0 km²) of it is land and 0.1 square miles (0.2 km²) of it is water. The total area is 10.47% water.

As of the census^GR2 of 2000, there were 4,871 people, 2,258 households, and 1,208 families residing in the borough. The population density was 6,308.6 people per square mile (2,442.5/km²). There were 2,656 housing units at an average density of 3,439.9/sq mi (1,331.8/km²). The racial makeup of the borough was 95.32% White, 3.24% African American, 0.12% Native American, 0.29% Asian, 0.23% from other races, and 0.80% from two or more races. Hispanic or Latino of any race were 0.72% of the population.

There were 2,258 households out of which 22.3% had children under the age of 18 living with them, 35.5% were married couples living together, 13.7% had a female householder with no husband present, and 46.5% were non-families. 41.8% of all households were made up of individuals and 21.9% had someone living alone who was 65 years of age or older. The average household size was 2.11 and the average family size was 2.88.

In the borough the population was spread out with 20.5% under the age of 18, 7.1% from 18 to 24, 27.1% from 25 to 44, 20.2% from 45 to 64, and 25.0% who were 65 years of age or older. The median age was 41 years. For every 100 females there were 81.4 males. For every 100 females age 18 and over, there were 77.1 males.

The median income for a household in the borough was $23,593, and the median income for a family was $31,699. Males had a median income of $30,093 versus $23,873 for females. The per capita income for the borough was $13,752. About 16.1% of families and 21.3% of the population were below the poverty line, including 36.2% of those under age 18 and 13.7% of those age 65 or over.

Charleroi is a namesake and Sister city of Charleroi, Belgium. The name is French for "Charles [the] King" (referring to King Charles II of Spain).

• Governor John K. Tener, a Republican, in office from 1911 to 1915
• Hardie Albright, actor
• Lisa Kirk, actress-singer
• Deborah Jeane Palfrey, a former Charleroi resident, Charleroi High School alumni organizer, and so-called "DC Madame" (see http://deborahjeanepalfrey.com/).
• Mitchell Paige, WWII Medal of Honor recipient

A large part of the plot of the alternate history novel The Two Georges, by Harry Turtledove and Richard Dreyfuss, takes place in Charleroi, Pennsylvania. In the alternate history of this book, North America remains part of the British Empire. Charleroi is described as a large coal-mining town filled with embittered coal miners of mainly Irish descent living under conditions of poverty, exploitation and pollution, who end up supporting radical underground political movements.

• Charleroi, Pennsylvania is at coordinates 40°08′17″N 79°54′05″W / 40.138088, -79.901333Coordinates: 40°08′17″N 79°54′05″W / 40.138088, -79.901333

v • d • e Municipalities and communities of Washington County, Pennsylvania
County seat: Washington
Cities	Monongahela | Washington
Boroughs	Allenport | Beallsville | Bentleyville | Burgettstown | California | Canonsburg | Centerville | Charleroi | Claysville | Coal Center | Cokeburg | Deemston | Donora | Dunlevy | East Washington | Elco | Ellsworth | Finleyville | Green Hills | Houston | Long Branch | Marianna | McDonald | Midway | New Eagle | North Charleroi | Roscoe | Speers | Stockdale | Twilight | West Alexander | West Brownsville | West Middletown
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CDPs	Baidland | Cecil-Bishop | Fredericktown-Millsboro | Gastonville | McGovern | McMurray | Thompsonville | Wickerham Manor-Fisher | Wolfdale
Communities	Condit Crossing | Eighty Four